World Congress on Biosensors 2014

World Congress on Biosensors 2014
Biosensors 2014

Thursday 27 September 2012

Just Published: Journal of Chromatography B


A new issue of this journal has just been published. To see abstracts of the papers it contains (with links through to the full papers) click here:
Selected papers from the latest issue:

Liquid chromatography–tandem mass spectrometry method for simultaneous determination of seven commonly used anticancer drugs in human plasma

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Jingya Zhou, Shouhong Gao, Feng Zhang, Bo Jiang, Qin Zhan, Fei Cai, Jingxian Li, Wansheng Chen
This paper describes the development and validation of a novel, general liquid chromatography–tandem mass spectrometry (LC–MS/MS) method for the simultaneous determination of cyclophosphamide, ifosfamide, irinotecan, etoposide, gemcitabine, carboplatin and pemetrexed concentrations in human plasma. Samples were prepared by two kinds of extraction method and analyzed using a gradient separation over an Atlantis T3-C18 column (2.1mm×100mm, 3μm, Waters). Positive electrospray ionization was employed as the ionization source. The mobile phase consisted of acetonitrile–water (0.1% formic acid and 10mM ammonium acetate) at a flow rate of 0.25mL/min. Linear coefficients of correlation were >0.992 for all analytes. The intra- and inter-day relative standard deviation across three validation runs over the entire concentration range was less than 9.2%, while the accuracy was within ±10.5%. The mean recovery of all the analytes ranged from 50.0 to 81.0%. This method was successfully applied to clinical samples from cancer patients.

Highlights

► We developed a novel, sensitive, reproducible, and accurate LC–MS/MS method. ► This method could simultaneous determination of seven anticancer drugs in human plasma. ► This new method was successfully applied to clinical samples from cancer patients.

Multi-detection of preservatives in cheeses by liquid chromatography–tandem mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Fabio Fuselli, Chiara Guarino, Alessandro La Mantia, Lucia Longo, Angelo Faberi, Rosa Maria Marianella
The incorrect use of preservatives in cheeses may compromise food safety and damage consumers. According to the law, more than one preservative may be contemporarily used in cheeses. So a method for their contemporary detection may be useful for both manufacturers and control agencies quality control. In this research a liquid chromatography–tandem mass spectrometric with electrospray ionization method for the multi-determination of seven preservatives (benzoic acid, citric acid, hexamethylenetetramine, lysozyme, natamycin, nisin and sorbic acid) in cheese was developed. The preservatives were contemporarily extracted from cheese by a single procedure, and analyzed by RP-LC/ESI-MS/MS (Ion Trap) in positive ionization mode, with single reaction monitoring (SRM) acquisition. Three sample types (hard, pasta filata and fresh cheese) were used for method evaluation. Recoveries were mostly higher than 90%; MDLs ranged from 0.02 to 0.26mgkg−1, and MQLs were included between 0.07 and 0.88mgkg−1. Due to matrix effect, quantitation was performed by referring to a matrix matched calibration curve, for each cheese typology. This method was also applied to commercial cheese samples, with good results. It appears fast, reliable and suitable for both screening and confirmation of the presence and quantitation of the preservatives in a single, multi-detection analysis.

Highlights

► An RP-HPLC–ESI-MS/MS based method was developed for the multi-determination of seven preservatives in three typologies of cheeses. ► The analytical strategy was evaluated in terms of accuracy, precision, limit of detection, and limit of quantification. ► Our method was applied to commercial cheese samples with good results.

Novel affinity purification of xanthine oxidase from Arthrobacter M3

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Yuran Zhang, Yu Xin, Hailin Yang, Ling Zhang, Xiaole Xia, Yanjun Tong, Yi Chen, Li Ma, Wu Wang
An affinity protocol for purification of xanthine oxidase (XOD) from Arthrobacter M3 was developed. The isolation procedure consisted of only three steps, ammonium sulfate precipitation, affinity extraction to exclude the major impurities, and the final refining procedure with DEAE ion-exchange chromatography for removal of minor contaminants. In this affinity preparation, guanine, an analogue of xanthine, was chosen as the affinity ligand, and was coupled with Sepharose 4B through spacers composed of epichlorohydrin and ethylenediamine. Crude protein has been run through ammonium sulfate precipitation and the affinity column, 99.1% of proteins were removed. After DEAE ion-exchange chromatography, the purity of the refined XOD was 97.5% by Native-PAGE analysis. The activity recovery of purified XOD (36.1%) was almost higher than that of other methods reported. Reducing SDS-PAGE analysis showed that the purified XOD (one band in Native-PAGE analysis) showed two polypeptides with the molecular weights ∼35kDa and ∼100kDa, respectively. The desorption constant K d and the theoretical maximum absorption Q max on the affinity medium were 3.0μg/ml and 2.2mg/g medium in absorption analysis.

Highlights

► A novel affinity protocol for the purification of xanthine oxidase is developed. ► Only three steps successfully purified xanthine oxidase. ► The most important step of this protocol is affinity chromatography. ► The mechanism relies on the affinity interaction between ligand and the enzyme. ► This method has advantage of fewer steps, better recoveries, and higher purity.

Development of a sensitive HPLC method to measure in vitro permeability of E- and Z-isomeric forms of thiosemicarbazones in Caco-2 monolayers

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Zufan Debebe, Sergei Nekhai, Meseret Ashenafi, David B. Lovejoy, Danuta S. Kalinowski, Victor R. Gordeuk, W. Malcolm Byrnes, Des R. Richardson, Pradeep K. Karla
In the current study, we developed a HPLC method to quantitatively measure the permeability of the BpT-based chelators, 2-benzoylpyridine 4-ethyl-3-thiosemicarbazone (Bp4eT) and 2-benzoylpyridine 4-allyl-3-thiosemicarbazone (Bp4aT), across human colorectal adenocarcinoma (Caco-2) monolayers as a model of gut absorption. In aqueous solution, Bp4eT and Bp4aT formed inter-convertible Z and E isomers that were resolved by HPLC. Peak area was linear with respect to chelator concentration. Acceptable within-day and between-day precision (<22%) and accuracy (85–115% of true values) were obtained over a range of 1.0–100μM for Bp4eT and 1.5–300μM for Bp4aT. Limits of detection were 0.3μM and 1μM for Bp4eT and Bp4aT, respectively, while corresponding limits of quantification were 1μM and 5μM. Both chelators showed significant ability to chelate iron in THP-1 cells using a calcein-based assay and no apparent cytotoxicity was observed within 24h. Ratios of the apical to basolateral and basolateral to apical transport for Bp4eT were 1.10 and 0.89 at 100μM and 300μM respectively, indicating equal bi-directional movement of the compounds. Similarly, ratios were 0.77 and 0.92 for Bp4aT, respectively. This study demonstrates that Bp4eT and Bp4aT can be efficiently transported through Caco-2 cells and can potentially be formulated for oral delivery.

Highlights

► We developed a sensitive HPLC method for assessment of BpT-E/Z isomers. ► We demonstrated effective iron chelation of BpT-iron chelators that inhibit HIV-1. ► We estimated the permeability profile of BpT-E/Z isomers in Caco2 monolayers. ► We anticipate that BpT chelators could hold promise as orally effective agents.

Identification of the urinary metabolites of glionitrin A in rats using ultra-performance liquid chromatography combined with quadrupole time-of-flight mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Soo Hyun Lee, Hyun Ok Yang, Hak Cheol Kwon, Byung Hwa Jung
Glionitrin A (GN A) is a new diketopiperazine disulfide with an aromatic nitro group, which is isolated from the coculture of an Aspergillus fumigatus fungal strain and a Sphingomonas bacterial strain. After intravenous administration of GN A in rats, 13 urinary metabolites of GN A were identified using ultra-performance liquid chromatography/quadrupole time-of-flight mass spectroscopy (UPLC–QTOP-MS) analysis in conjunction with data processing programs such as MetaboLynx™ and MassFragnent™. Reduction, nitro-reduction and hydration were the primary metabolic processes affecting GN A in vivo, followed by demethylation or oxidative deamination to alcohol, as well as cysteine, glycine, glucuronide or sulfate conjugation. The metabolite resulting from reduction was found to be a molecule with a dithiol group, and the metabolite made by nitro reduction was found to be an aromatic amine corresponding to GN A. Both of these products may have pharmacological or toxicological activity, which is valuable information in terms of using GN A as a lead compound. In addition, this work showed that UPLC–QTOP-MS analysis coupled with efficient data processing programs is useful for rapid and reliable characterization of GN A metabolites in vivo.

Highlights

► After intravenous administration of GN A in rats, urinary metabolites of GN A were identified. ► Metabolite identification was performed using UPLC–QTOP-MS analysis in conjunction with data processing programs. ► Reduction, nitro-reduction and hydration were the primary metabolic processes affecting GN A in vivo. ► Demethylation, oxidative deamination to alcohol and conjugations were also included in GN A metabolism.

On-line sample concentration and determination of cationic alkaloids in human plasma by micelle to solvent stacking in capillary zone electrophoresis

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Shuaihua Zhang, Ruiyang Ma, Xiumin Yang, Chun Wang, Zhi Wang
A sensitive method for the determination of three cationic alkaloids (berberine, palmatine and jatrorrhizine) from human plasma samples was developed by micelle to solvent stacking (MSS) in capillary zone electrophoresis (CZE). In MSS, the sample preconcentration mainly relies on the reversal in the effective electrophoretic mobility of the analytes at the boundary zone between the sample and CZE background solution (BGS). Under the optimized conditions, the sensitivity enhancement factors achieved in terms of corrected peak area were in the range from 47 to 53 for the alkaloids. The limits of detection (LODs) (S/N=3) for berberine, palmatine and jatrorrhizine were 0.01, 0.01 and 0.02μg/mL, respectively. The intraday (n =6) and interday repeatabilities (n =12) expressed as the relative standard deviations (RSDs) were less than 6.9% in terms of peak height and less than 7.3% in terms of corrected peak area, respectively. The recoveries of the method for the three alkaloids were in the range of 95.9–101.5% with peak height as the quantitative signal, and 92.6–103.6% with corrected peak area as the quantitative signal, respectively. The MSS-CZE method proved to be suitable for the analysis of the alkaloids in human plasma samples.

Highlights

► On-line sample concentration and analysis of some cationic alkaloids in human plasma. ► Micelle to solvent stacking in capillary zone electrophoresis. ► High sensitivity and good recovery.

Generic and rapid determination of veterinary drug residues and other contaminants in raw milk by ultra performance liquid chromatography–tandem mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Jia Zhan, Xue-jun Yu, Ying-ying Zhong, Zai-ting Zhang, Xiao-mei Cui, Jin-feng Peng, Rui Feng, Xiao-tao Liu, Yan Zhu
A generic, rapid and simple analytical method able to identify 255 veterinary drug residues and other contaminants in raw milk had been developed. The method was based on two-step simple precipitation and ultra performance liquid chromatography coupled with electrospray ionization and tandem mass spectrometry (UPLC–ESI–MS/MS) operating both in positive and negative multiple reaction mode (MRM). For most of the target analytes, the optimized pretreatment processes led to no significant interference on analysis from complicated sample matrix. For quantification, matrix-fortified calibration curves were performed to compensate for the matrix effect and loss in sample preparation. Competent linearity was found for over 90% of target compounds with linear regression coefficients (R) higher than 0.99. Detection limits ranged from 0.05 to 10μg/kg. Average recoveries spiked into raw milk were in the range from 63% to 141% with associated RSD values from 1% to 29% under the selected conditions. The method had been validated for its extraction sensitivity, linearity, recoveries and precision. The results clearly demonstrated the feasibility of the approach proposed. Application of this method, which improved efficiency and coverage of residues, would imply a drastic reduction of both effort and time in routine monitoring programs.

Highlights

► First, the proposed method was generic for a wide range polarity compounds. ► Second, the method, with only two steps, was rapid and straightforward. ► Third, the way to remove water in milk for concentration was novelty. ► Finally, this kind of method is urgently needed in dairy plants.

Aqueous normal phase liquid chromatography coupled with tandem time-of-flight quadrupole mass spectrometry for determination of zanamivir in human serum

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Jing Ge, Fengmao Liu, Eric H. Holmes, Gary K. Ostrander, Qing X. Li
An aqueous normal phase (ANP) liquid chromatography coupled with a hybrid quadrupole time-of-flight mass spectrometry (ANP-LC-micrOTOFQ) method was used for the determination of zanamivir in human serum. Zanamivir was extracted with methanol from protein-precipitated human serum samples and further purified with SCX solid-phase extraction cartridges. Scherzo SM-C18, Agilent Zorbax SB-Aq, Cogent Diamond Hydride, Cogent Bidentate and Luna HILIC columns were compared and optimized for the retention and separation of zanamivir and the Luna HILIC and Diamond Hydride columns exhibited the best retention of zanamivir. The former provided a shorter retention time, a sharper peak and relatively high sensitivity, whereas the latter exhibited a longer retention time and less matrix interference. The analytical range of the calibration curve was between 5 and 1000ng/mL.

Highlights

► Aqueous normal phase chromatography was studied for the separation of zanamivir in human sera. ► Five different columns were compared for the capability to retain zanamivir. ► Effects of mobile phase constituents on the retention time were examined. ► The Diamond Hydride column was the most effective to retain zanamivir and avoid matrix effects.

Development and validation of a rapid capillary zone electrophoresis method for determining charge variants of mAb

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Ying Shi, Zhen Li, Yuanbiao Qiao, Jun Lin
This work aimed to develop a rapid capillary zone electrophoresis (CZE) method to provide abundant purity and identity information of monoclonal antibodies. The CZE running buffer system was optimized to be 20mM acetate–acetic acid (pH 6.0) together with the co-addition of 0.3% polyethylene oxide (PEO) and 2mM triethylenetetramine (TETA), which was further tested with advantages on the peak resolution improvements. The conditioning period was scheduled to 1min for both 0.1M HCl and CZE running buffer to reduce total separation time. Additionally, the applied voltage and effective separation length were optimized at 30kV and 20cm separately. Compared with the method reported by Yan [1], this newly developed method showed a higher resolution in separating the two unknown basic peaks by testing monoclonal antibody sample (mAb1). The further validation results showed that for all five of charge isoform peaks of test mAb1, repeatability, intraday and interday precision had a RSD less than 0.58% for migration time and less than 3.18% for corrected area percent. The correlation coefficients of more than 0.98 for all peaks also demonstrated the good linearity for the method. In addition to the application of distinguishing intact antibody from C-terminal Lys variants, the method also has advantage in separating the Fab, Fc and intact antibody-relevant substances quickly, which facilitated the rough evaluation of papain induced digestion.

Highlights

► We prepared a simple CZE running buffer. ► We developed and optimized a CZE method in dynamically coated capillary. ► We performed fast separation in less than 5min with high resolution.

Simultaneous determination of azelastine and its major metabolite desmethylazelastine in human plasma using high performance liquid chromatography–tandem mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Wuyi Zha, Linyee Shum
A selective and sensitive high performance liquid chromatography–tandem mass spectrometric method was developed for the analysis of azelastine and its major metabolite, desmethylazelastine, in human plasma. Azelastine-13C, d3 was used as internal standard. Azelastine, desmethylazelastine and the internal standard were extracted by a liquid–liquid extraction method and separation was performed under isocratic chromatographic condition. An abnormal signal loss issue for desmethylazelastine during method development was investigated and resolved. The developed method was precise and reproducible as shown by good intraday assay and interday assay precision (CV%≤12.8%). The calibration curve was linear over a range of 10.0/10.0–1000/200pg/mL for azelastine/desmethylazelastine. The method was successfully applied to a pilot bioequivalence study subsequently.

Highlights

► LC–MS/MS method for simultaneous quantitation of azelastine and desmethylazelastine. ► Low LOQ of 10pg/mL for both compounds were achieved. ► An abnormal signal loss issue for desmethylazelastine was investigated and resolved.

Simultaneous determination of eight corticosteroids in bovine tissues using liquid chromatography–tandem mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Ádám Tölgyesi, Virender K. Sharma, Szabolcs Fekete, Dóra Lukonics, Jenő Fekete
This paper describes a newly developed method for the simultaneous determination of eight corticosteroid residues in bovine muscle, liver and kidney samples using liquid chromatography–tandem mass spectrometry (LC–MS/MS). The determination of methylprednisone, the main metabolite of methylprednisolone, in bovine tissues using LC–MS/MS is carried out for the first time. The method development demonstrates that the pH is important in optimizing the sample preparation. Tests performed using different solid-phase extraction (SPE) cartridges were enabled to produce conditions for reducing the matrix effects (ion suppression and enhancement) of analysis. Acidic condition and mixed-mode cation exchange SPE columns resulted in the most suitable clean-up for muscle and liver, and also yielded acceptable results for kidney. The enhanced sample clean-up resulted in excellent clear baselines of ion transitions, and therefore, a higher delta electron multiplier voltage (ΔEMV) could be set in the MS/MS detector. The application of 500V of ΔEMV improved the signal responses, however, the noise level did not change, and consequently, the overall sensitivity and analytical limits (limit of detection, limit of quantification) could be enhanced. In the HPLC separation, the recently introduced Kinetex phenyl-hexyl core–shell type column was used that enabled baseline separation for dexamethasone and its β-epimer, betamethasone. Dexamethasone and betamethasone were eluted within 12min and such reduced retention, obtained with core–shell HPLC type column, further enhanced the sensitivity. The method was validated according to the European Union (EU) 2002/657/EC Decision; the studied parameters met the EU standards. The decision limits and limit of detections were calculated in each matrix for all corticosteroids and varied from 0.01 to 13.3μg/kg and from 0.01 to 0.1μg/kg, respectively.

Highlights

► A new LC–MS/MS method is developed for corticosteroids in tissue samples. ► Acidic pH control and mixed-mode SPE cartridges are essential for sample clean-up. ► Corticosteroid epimers can be separated simultaneously using Kinetex HPLC column. ► The enhanced clean-up and LC–MS/MS separation improved the analytical limits. ► The method is successful in analyzing dexamethasone in incurred samples.

Validation of a chiral liquid chromatography–tandem mass spectrometry method for the determination of pantoprazole in dog plasma

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Meixia Chen, Yu Xia, Zhiyu Ma, Liang Li, Dafang Zhong, Xiaoyan Chen
Pantoprazole (PAN), a selective proton pump inhibitor, is used clinically as a racemic mixture for the treatment of acid-related gastrointestinal disorders. To investigate its stereoselective pharmacokinetics, a chiral liquid chromatography–tandem mass spectrometry method was developed and validated to determine the pantoprazole enantiomers in dog plasma. After liquid–liquid extraction, a baseline resolution of enantiomers was achieved on an ovomucoid column using the mobile phase of methanol:acetonitrile:10mM ammonium formate (pH 7) (10.4:2.6:87, v/v/v) at 30°C within 10min. Stable isotopically labeled (+)-d3-pantoprazole and (−)-d3-pantoprazole were used as internal standards. Acquisition of mass spectrometric data was performed in multiple reaction monitoring mode via positive atmospheric pressure chemical ionization. The method was linear in the concentration range of 20.0–10,000ng/mL for each enantiomer using 25μL of dog plasma. The lower limit of quantification (LLOQ) for each enantiomer was 20.0ng/mL. Intra- and inter-day precision ranged from 3.2% to 10.3% for (+)-pantoprazole and 3.7–10.0% for (−)-pantoprazole. Accuracy varied from −1.4% to −0.2% for (+)-pantoprazole and −1.6% to 0.8% for (−)-pantoprazole. The validated method was applied successfully for stereoselective pharmacokinetic studies of racemic pantoprazole.

Highlights

► A chiral LC–MS/MS method was validated to quantify pantoprazole enantiomers. ► Separation was performed on an ovomucoid protein column using MS compatible mobile phases. ► Baseline resolution within 10min leads to a reduction in the overall analysis time.

Rapid resolution liquid chromatography (RRLC) analysis of amino acids using pre-column derivatization

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B, Volume 906
Xiaoli Zhang, Tong Zhao, Ting Cheng, Xiaoyan Liu, Haixia Zhang
A rapid resolution liquid chromatography (RRLC) method was developed for the simultaneous determination of 23 amino acids in rat serum after pre-column derivatization with 2,4-dinitrofluorobenzene (DNFB). The amino acid derivatives were separated on an Agilent Zorbax Eclipse Plus C18 (4.6mm×50mm, 1.8μm) column at 45°C. Ultraviolet (UV) detection was set at 360nm. Good separation of 23 amino acids was achieved within 10min with a ternary gradient elution of mobile phase at a flow rate of 1.5mLmin−1. Calibration curves were linear over the range from 1 to 500μmolL−1 with coefficients 0.9962 or better for each amino acid. The lower limits of quantification (LLOQ) of all 23 amino acids were 1μmolL−1 with signal-to-noise (S/N) ratio ≥4. Intra- and Inter-day precisions, expressed as relative standard deviation (RSD) percentages, were ranged from 0.32% to 3.09% and 0.67% to 5.82%, respectively. Finally, it was successfully applied to the determination of amino acids in rat serum with recoveries ranged from 90.8% to 106.0% and RSD percentages ranged from 1.78% to 4.68%, respectively. The results showed that the proposed method provided a shorter elution time, better resolution and sharper peak shapes for all amino acids. Compared with the conventional high performance liquid chromatography (HPLC) methods, even some ultra-performance liquid chromatography tandem mass spectrometry (UPLC–MS/MS), the established RRLC method was superior performance.

Highlights

► The RRLC method was the first time used for amino acids detection. ► Compared with common HPLC and some UPLC, the RRLC was superior performance. ► The reduced solvent consumption was friendly to environment protection. ► The RRLC based on UV detection was economic and available in common laboratories.

Capillary electrophoresis to quantitate gossypol enantiomers in cotton flower petals and seed

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B
Sergey Vshivkov, Egor Pshenichnov, Zamira Golubenko, Alik Akhunov, Shadman Namazov, Robert D. Stipanovic
Gossypol is a toxic compound that occurs as a mixture of enantiomers in cotton plant tissues including seed and flower petals. The (-)-enantiomer is more toxic to non-ruminant animals. Efforts to breed cottonseed with a low percentage of (-)-gossypol requires determination of the (+)- to (-)-gossypol ratio in seed and flower petals. We report a method to quantitatively determine the total gossypol and percent of its enantiomers in cotton tissues using high performance capillary electrophoresis (HPCE). The method utilizes a borate buffer at pH 9.3 using a capillary with internal diameter of 50μm, effective length of 24.5cm, 15kV and cassette temperature of 15°C. This method provides high accuracy and reproducible results with a limit of detection of the individual enantiomers of less than 36ng/mL providing base line separation in less than 6minutes.

Highlights

► Gossypol occurs as a mixture of enantiomers in cottonseed. ► (-)-Gossypol is more toxic to non-ruminant animals. ► Plant breeders are developing plants with a low percent of (-)gossypol. ► A capillary electrophoresis method was developed to quantitate the enantiomers. ► Breeders can use this method to select plants with the low (-)gossypol seed trait.

Characterization and identification of alanine to serine sequence variants in an IgG4 monoclonal antibody produced in mammalian cell lines

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B
Jinmei Fu, Jacob Bongers, Li Tao, Dan Huang, Richard Ludwig, Yunping Huang, Yueming Qian, Jonathan Basch, Joel Goldstein, Ramji Krishnan, Li You, Zheng Jian Li, Michael J. Grace, Reb J. Russell
Low levels of alanine to serine sequence variants were identified in an IgG4 monoclonal antibody by ultra/high performance liquid chromatography and tandem mass spectrometry. The levels of the identified sequence variants A183S and A152S, both in the light chain, have been determined to be 7.8-9.9% and 0.5-0.6%, by extracted ion currents of the tryptic peptides L16 and L14, respectively. The A183S variant was confirmed through tryptic map spiking experiments using synthetic peptide, SDYEK, which incorporated Ser at the position of native Ala in the tryptic peptide L16. Both mutations were also observed by endoproteinase Asp-N peptide mapping. The variant level of A183S was also quantified by LC-UV with detection at 280nm and fluorescence detection of tyrosine residues on the tryptic peptides. The results from LC-MS, UV, and fluorescent detection are in close agreement with each other. The levels of the sequence variants are comparable among the antibody samples manufactured at different scales as well as locations, indicating that the variants’ levels are not affected by manufacture scale or locations. DNA sequencing of the master cell bank revealed the presence of mixed bases at position 183 encoding both wild and mutated populations, whereas bases encoding the minor sequence variant at position152 were not detected. The root cause for A152S mutation is not yet clearly understood at this moment.

Highlights

► Alanine to serine sequence variants were identified in an IgG4 monoclonal antibody by LC/MS/MS. ► The sequence variants were confirmed by use of synthetic peptide. ► DNA sequencing of the mater cell bank revealed one variant was caused by mutation at the DNA level.

Simultaneous determination of morinidazole, its N-oxide, sulfate, and diastereoisomeric N+-glucuronides in human plasma by liquid chromatography–tandem mass spectrometry

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B
Ruina Gao, Dafang Zhong, Ke Liu, Yu Xia, Rongwei Shi, Hua Li, Xiaoyan Chen
Morinidazole is a new third-generation 5-nitroimidazole antimicrobial drug. To investigate the pharmacokinetic profiles of morinidazole and its major metabolites in humans, a liquid chromatography–tandem mass spectrometry method was developed and validated for simultaneous determination of morinidazole, its N-oxide metabolite (M4-1), a sulfate conjugate (M7), and two diastereoisomeric N +-glucuronides (M8-1 and M8-2) in human plasma. A simple acetonitrile-induced protein precipitation was employed to extract five analytes and internal standard metronidazole from 50 μL human plasma. To avoid the interference from the in-source dissociation of the sulfate and achieve the baseline-separation of diastereoisomeric N +-glucuronides, all the analytes were separated from each other with the mobile phase consisting of 10mM ammonium formate and acetonitrile using gradient elution on a Hydro-RP C18 column (50 mm × 2 mm, 4 μm) with a total run time of 5 min. The API 4000 triple quadrupole mass spectrometer was operated under the multiple reaction-monitoring mode using the electrospray ionization technique. The developed method was linear in the concentration ranges of 10.0ng/mL to 12000ng/mL for morinidazole, 1.00ng/mL to 200ng/mL for M4-1, 2.50ng/mL to 500ng/mL for M7, 3.00ng/mL to 600ng/mL for M8-1, and 10.0ng/mL to 3000ng/mL for M8-2. The intra- and inter-day precisions for each analyte met the accepted value. Results of the stability of morinidazole and its metabolites in human plasma were also presented. The method was successfully applied to the clinical pharmacokinetic studies of morinidazole injection in healthy subjects, patients with moderate hepatic insufficiency, and patients with severe renal insufficiency, respectively.

Highlights

► Simultaneously determine morinidazole and its four metabolites in human plasma. ► Gradient elution was used to obtain the resolution of two N+-glucuronide isomers. ► The potential interference from the in-source dissociation of the conjugates was avoided. ► The method was applied to clinical pharmacokinetic studies of morinidazole injection.

Short-incubation mass spectrometry assay for lysosomal storage disorders in newborn and high-risk population screening

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B
Thomas P. Mechtler, Thomas F. Metz, Hannes G. Müller, Katharina Ostermann, Rene Ratschmann, Victor R. De Jesus, Bori Shushan, Joseph M. Di Bussolo, Joseph L. Herman, Kurt R. Herkner, David C. Kasper
The interest in early detection strategies for lysosomal storage disorders (LSDs) in newborns and high-risk population has increased in the last years due to the availability of novel treatment strategies coupled with the development of diagnostic techniques. We report the development of a short-incubation mass spectrometry-based protocol that allows the detection of Gaucher, Niemann-Pick A/B, Pompe, Fabry and mucopolysaccharidosis type I disease within four hours including sample preparation from dried blood spots. Optimized sample handling without the need of time-consuming offline preparations, such as liquid-liquid and solid-phase extraction, allows the simultaneous quantification of five lysosomal enzyme activities using a cassette of substrates and deuterated internal standards. Applying incubation times of 3h revealed in intra - day CV% values ranging from 4% to 11% for all five enzyme activities, respectively. In a first clinical evaluation, we tested 825 unaffected newborns and 16 patients with LSDs using a multiplexed, turbulent flow chromatography–ultra high performance liquid chromatography–tandem mass spectrometer assay. All affected patients were identified accurately and could be differentiated from non-affected newborns. In comparison to previously published two-day assays, which included an overnight incubation, this protocol enabled the detection of lysosomal enzyme activities from sample to first result within half a day.

Highlights

► We report a short-incubation mass spectrometry-based protocol for lysosomal enzymes. ► Optimized sample handling and online clean-up allowed a 4h analysis. ► Up to 5 lysosomal enzyme activities are analyzed simultaneously from dried blood spots. ► Method validation was performed under routine clinical laboratory environment.

Determination of five di-(2-ethylhexyl)phthalate metabolites in urine by UPLC-MS/MS, markers of blood transfusion misuse in sports

27 September 2012, 09:32:50
Publication year: 2012
Source:Journal of Chromatography B
Núria Monfort, Rosa Ventura, Georgina Balcells, Jordi Segura
Di-(2-ethylhexyl)phthalate (DEHP) is the most commonly used plasticizer for polyvinyl chloride, which is found in a large variety of products, including most of the bags used for blood storage because of its protective role on erythrocytes survival. DEHP metabolites have been recently proposed as markers of the misuse of blood transfusion in athletes. In this study, a method to quantify the main five DEHP metabolites in urine has been developed: mono-(2-ethylhexyl)phthalate (MEHP), mono-(2-ethyl-5-hydroxyhexyl)phthalate (MEHHP), mono-(2-ethyl-5-oxohexyl)phthalate (MEOHP), mono-(2-ethyl-5-carboxypentyl)phthalate (5cx-MEPP), and mono-(2-carboxymethylhexyl)phthalate (2cx-MMHP). The method involved an enzymatic hydrolysis with β-glucuronidase from Escherichia coli followed by an acidic extraction with ethyl acetate. The hydrolyzed extracts were analysed by ultraperformance liquid chromatography tandem mass spectrometry. Isotope labelled MEHP, MEOHP and 5cx-MEPP were used as internal standards. Analysis of all the metabolites was achieved in a total run time of 10min, using a C18 column and a mobile phase containing deionized water and acetonitrile with formic acid, with gradient elution at a flow-rate of 0.6mLmin−1. Detection of the compounds was performed by multiple reaction monitoring, using electrospray ionization in positive and negative ion modes. The method was validated for quantitative purposes. Extraction recoveries were greater than 90% and the limits of quantitation ranged from 1.2 to 2.6ngmL−1. Intra-day precisions were better than 8% for all metabolites while inter-assay precisions were better than 12%. Concentrations of DEHP metabolites were measured in a control group (n=30, subjects reflecting the common environmental DEHP exposure), and in sportsmen (n=464), to evaluate population distribution exposure to DEHP. Additionally, threshold concentrations indicating outliers of common exposure for DEHP metabolites are proposed.

Highlights

► Di-(2-ethylhexyl)phthalate (DEHP) is the most commonly used plasticizer for PVC ► DEHP metabolites have been proposed as markers of the misuse of blood transfusion ► A method to quantify five DEHP metabolites has been developed and validated ► Cutoff concentrations were proposed to determine suspicions of a possible transfusion ► The method is proposed as screening test for transfusion detection in doping control


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